Chris Evans
Steve Rogers / Captain America
Acting
Samuel L. Jackson
Nick Fury
Acting
Scarlett Johansson
Natasha Romanoff / Black Widow
Acting
Robert Redford
Alexander Pierce
Acting
Sebastian Stan
Bucky Barnes / Winter Soldier
Acting
Anthony Mackie
Sam Wilson / Falcon
Acting
Cobie Smulders
Maria Hill
Acting
Frank Grillo
Brock Rumlow
Acting
Maximiliano Hernández
Jasper Sitwell
Acting
Emily VanCamp
Kate / Agent 13
Acting
Hayley Atwell
Peggy Carter
Acting
Toby Jones
Dr. Arnim Zola
Acting
Stan Lee
Smithsonian Guard
Writing
Callan Mulvey
Jack Rollins
Acting
Jenny Agutter
Councilwoman Hawley
Acting
Bernard White
Councilman Singh
Acting
Alan Dale
Councilman Rockwell
Acting
Chin Han
Councilman Yen
Acting
Garry Shandling
Senator Stern
Acting
Georges St-Pierre
Georges Batroc
Acting
Salvator Xuereb
French Pirate #1
Acting
Brian Duffy
French Pirate #2
Crew
Zack Duhame
Engine Pirate
Crew
Adetokumboh M'Cormack
French Radio Pirate
Acting
Christopher George Sarris
Skinny Steve
Acting
Aaron Himelstein
Launch Tech #1
Acting
Allan Chanes
Launch Tech #2
Acting
Joe Russo
Dr. Fine
Directing
Christopher Markus
SHIELD Interrogator #1
Writing
Stephen McFeely
SHIELD Interrogator #2
Writing
Pat Healy
Scientist #1
Acting
Ed Brubaker
Scientist #2
Writing
D.C. Pierson
Apple Employee
Acting
Danny Pudi
Com Tech #1
Acting
Bernie Zilinskas
Com Tech #2
Acting
Branka Katić
Renata
Acting
Angela Russo-Otstot
Garcia
Production
Jon Sklaroff
Charlie XO
Acting
Chad Todhunter
Charlie Weapons Tech
Acting
Abigail Marlowe
SHIELD Tech
Acting
Jeremy Maxwell
Lead SHIELD Pilot
Acting
Emerson Brooks
Senior SHIELD Agent
Acting
Evan Parke
SHIELD Agent
Acting
Ricardo Chacon
Strike SGT. #1
Acting
Griffin M. Allen
Strike SGT. #2
Acting
Ann Russo
Strike Agent
Acting
Joe Rosalina
Strike Agent
Acting
Michael Debeljak
Strike Agent
Acting
Eddie J. Fernandez
Strike Agent
Crew
Jody Hart
25ᵗʰ Floor Strike Agent
Acting
Steven Culp
Scudder
Acting
Derek Hughes
Human Resources Executive
Acting
Wendy Hoopes
Doctor
Acting
Ethan Rains
Lead EMT
Acting
Dominic Rains
CIA Instructor
Acting
Charles Wittman
Capitol Hill Police
Acting
Andy Martinez, Jr.
Capitol Hill Police
Acting
Michael De Geus
FBI Agent
Acting
Terence O'Rourke
FBI Agent
Acting
Anne Grimenstein
Committee Member
Acting
Dante Rosalina
Little Boy in the Smithsonian
Acting
Robert Clotworthy
Fury Car Voice (voice)
Acting
June Christopher
SHIELD Computer (voice)
Acting
Gary Sinise
The Smithsonian Narrator (voice)
Acting
Henry Goodman
Dr. List (uncredited)
Acting
Dean Barlage
SHIELD Agent (uncredited)
Acting
Joel Thingvall
Museum Visitor (uncredited)
Acting
Thomas Kretschmann
Baron Wolfgang von Strucker (uncredited)
Acting
Elizabeth Olsen
Wanda Maximoff / Scarlet Witch (uncredited)
Acting
Nestor Serrano
Committee General (uncredited)
Acting
Aaron Taylor-Johnson
Pietro Maximoff / Quicksilver (uncredited)
Acting
Joss Whedon
Man on Escalator in Museum (uncredited)
Writing
James Lewis
Smithsonian Museum Visitor
Acting